Probably the most numerous make of covered hopper ever (happy to be corrected)
I'd stake my money on the most numerous being either the Pullman Standard 4750 cubic foot cars that came a few years later than the 4427's, or the ACF Centerflow 4650 cubic foot cars. These two cars would represent the two most common designs on the rails from the early 70's through the bump in allowable gross rail load that happened in the latter part of the 90's.
I don't know exactly where to find the data for all cars, but
Tangent (an HO manufacturer) has a historical blurb on the 4750's that says they were the most produced car of this type. Gorgeous models, I wish we had something of this caliber in O scale.
As to whether the 4427's are still in use today, it's very likely that some are still running around. Although they would be right in the time frame when their service life in non-rebuilt form would expire. I can say that I saw a few in use when I still lived in Denver, probably in the 2010-2015 period. I left Denver at the end of 2015, so it was before then. The seven years in between is right on the cusp of the service life expiration, which is either 45 or 50 years from build date. So they may have come off the rails in the meantime. No matter what, most if not all 4427's would have been sold off from the class 1 carriers and be in service with secondhand owners like railcar leasing groups. I just checked some photo sites, there are pictures of 4427's in limited use up to as recently as June of this year. So they can still be found occasionally.
By the way, the roof walk extension brace at the "A" end (non brakewheel end) of the car needs reattachement. This is a common part to come loose, it would be prudent to check the Atlas 5161 cu. ft. hoppers for the same issue.
I'm nearly out of FNG so might pick a bottle of this up next.
You might consider getting the big 5kg jug of Navy Grey if you are going continue using it. You do enough printing that I doubt it would expire on you. It's a bit cheaper in bulk than in the 1kg bottles.
It's high cubes and tanks I'm in need of and most tank cars are poor renditions with over thick hand rails and poor joint lines in the tank itself.
Given what I understand about your era interests and your evolving sense of pragmatism, I think you might want to reconsider some of the Atlas tank cars. This is the Atlas 17.6k gallon car, frequently used for corn syrup service. But adaptable to other ladings as well.
I think the walkways and steps could use a bit of help, possibly the end-to-body join as well. But I think they present fairly well. Of course, getting them in the UK might tip the balance in favor of making your own.
Riveted tanks like Jason mentions would have gone out of fashion by the 80's, at least in common usage. That doesn't mean you couldn't use the ends if they were the right size. Picking a size and shape is tricky though, I find the variety of tank cars and detailing a bit overwhelming. There are so many types and uses, and corresponding sizes, that I find it hard to know which one's I should be aiming to model.
Jim